Photoelectrochemical comproportionation of pre-treated PET plastics and CO2 to formate [0.03%] 经预处理的PET塑料和二氧化碳光化学共合成甲酸
Yongpeng Liu,Celine Wing See Yeung,Erwin Reisner Yongpeng Liu
Pairing plastic waste reforming and carbon dioxide (CO2) utilisation to produce chemical energy carriers provides an attractive means to mitigate waste and create value, but challenges persist in achieving selective product formation, separ...
Craig Burdis,Romain Tort,Anna Winiwarter et al. Craig Burdis et al.
To introduce the potential for tuneability of the cathode in lithium mediated ammonia synthesis, we report a carbon cathode which produces ammonia at a faradaic efficiency of 37%. This provides a basis to optimise properties of carbon elect...
Pekka Peljo,Claire Villevieille,Hubert H Girault Pekka Peljo
This article aims to present the redox aspects of lithium-ion batteries both from a thermodynamic and from a conductivity viewpoint. We first recall the basic definitions of the electrochemical potential of the electron, and of the Fermi le...
Deep learning for augmented process monitoring of scalable perovskite thin-film fabrication [0.03%] 基于深度学习的钙钛矿薄膜规模化加工的增强型过程监控技术
Felix Laufer,Markus Götz,Ulrich W Paetzold Felix Laufer
Reproducible large-area fabrication is one of the remaining challenges for the commercialization of perovskite photovoltaics. Imaging methods augmented with deep learning (DL) enable in-line detection of spatial or temporal inconsistencies ...
Probing ionic conductivity and electric field screening in perovskite solar cells: a novel exploration through ion drift currents [0.03%] 探究钙钛矿太阳能电池中的离子电导和电场屏蔽:通过离子漂移电流进行的新探索
Matthias Diethelm,Tino Lukas,Joel Smith et al. Matthias Diethelm et al.
It is widely accepted that mobile ions are responsible for the slow electronic responses observed in metal halide perovskite-based optoelectronic devices, and strongly influence long-term operational stability. Electrical characterisation m...
A spiro-type self-assembled hole transporting monolayer for highly efficient and stable inverted perovskite solar cells and modules [0.03%] 高效稳定的倒置钙钛矿太阳能电池和组件的螺环型自组装空穴传输单分子层
Xianfu Zhang,Botong Li,Shaochen Zhang et al. Xianfu Zhang et al.
Self-assembled monolayers (SAMs) have significantly contributed to the advancement of hole transporting materials (HTMs) for inverted perovskite solar cells (PSCs). However, uneven distribution of SAMs on the substrate largely decreases the...
Techno-economic assessment of different small-scale electrochemical NH3 production plants [0.03%] 不同规模小型电化学NH3生产厂的技术经济评估
Boaz Izelaar,Mahinder Ramdin,Alexander Vlierboom et al. Boaz Izelaar et al.
Electrochemical ammonia synthesis via the nitrogen reduction reaction (NRR) has been poised as one of the promising technologies for the sustainable production of green ammonia. In this work, we developed extensive process models of fully i...
Distinguishing bulk redox from near-surface degradation in lithium nickel oxide cathodes [0.03%] 区分锂镍氧化物正极中的主体氧化还原与近表面降解
Lijin An,Jack E N Swallow,Peixi Cong et al. Lijin An et al.
Ni-rich layered oxide cathodes can deliver higher energy density batteries, but uncertainties remain over their charge compensation mechanisms and the degradation processes that limit cycle life. Trapped molecular O2 has been identified wit...
Ultra-uniform perovskite crystals formed in the presence of tetrabutylammonium bistriflimide afford efficient and stable perovskite solar cells [0.03%] 含四丁基氨基双三氟甲anesulfonimide的超均匀钙钛矿单晶及高效稳定钙钛矿太阳能电池
Jaekeun Lim,Alwani Imanah Rafieh,Naoyuki Shibayama et al. Jaekeun Lim et al.
Compositional engineering of organic-inorganic metal halide perovskite allows for improved optoelectrical properties, however, phase segregation occurs during crystal nucleation and limits perovskite solar cell device performance. Herein, w...
Operando Fe dissolution in Fe-N-C electrocatalysts during acidic oxygen reduction: impact of local pH change [0.03%] 酸性条件下Fe-N-C电催化剂进行氧还原时的原位铁溶解:局部pH变化的影响
Angus Pedersen,Kavita Kumar,Yu-Ping Ku et al. Angus Pedersen et al.
Atomic Fe in N-doped C (Fe-N-C) catalysts provide the most promising non-precious metal O2 reduction activity at the cathodes of proton exchange membrane fuel cells. However, one of the biggest remaining challenges to address towards their ...