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Two-Lever Design Rule for High-Entropy Oxide Oxygen Carriers: Minimize Spin Polarization, Maximize Fe-O-Ni Covalency

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What is missing in high-entropy oxide (HEO) oxygen carrier design is an actionable rule that links composition to redox performance. We advance a two-lever principle─decrease spin polarization and increase Fe-O-Ni covalency─that lowers the oxygen-vacancy for... ...