Gradient Polarization Induces Three-Dimensional Asymmetric Electron Distribution in Covalent Organic Frameworks for Dramatically Enhanced Photocatalytic Overall Nitrogen Fixation
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Constructing a donor-acceptor (D-A)-based covalent organic frameworks (COFs) is an effective approach to enhance photocatalytic efficiency, yet the spatial conformation imposes inherent trade-offs between in-plane and interplane carrier transport. Here, we pre... ...
