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Marine pollution bulletin. 2024 Feb:199:115931. doi: 10.1016/j.marpolbul.2023.115931 Q14.92025

Spatial distribution characteristics of perfluoroalkyl substances in bulk and grain size fractionated sediments in Shenzhen Bay

深圳湾沉积物中全氟烷基物质的空间分布特征bulk和粒径分级样品中的分布特性 翻译改进

Haoshuai Li  1, Zimin Wang  1, Yang Zhou  2, Cui Shi  3, Huayang Gan  2, Fang Chen  4, Lei Xing  5, Danxu Guo  1, Longhai Zhu  6, Nan Wang  7, Shuhong Fang  8, Rui Bao  9

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作者单位

  • 1 Frontiers Science Center for Deep Ocean Multispheres and Earth System, and Key Laboratory of Marine Chemistry Theory and Technology, Ministry of Education, Ocean University of China, Qingdao 266100, China; Laboratory for Marine Ecology and Environmental Science, Qingdao National Laboratory for Marine Science and Technology, Qingdao 266061, China.
  • 2 Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou), Guangzhou 5111458, China.
  • 3 Shenzhen Branch of China National Offshore Oil Corporation Limited, Shenzhen 518000, China.
  • 4 Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou), Guangzhou 5111458, China. Electronic address: Zhchenfang66@21cn.com.
  • 5 Frontiers Science Center for Deep Ocean Multispheres and Earth System, and Key Laboratory of Marine Chemistry Theory and Technology, Ministry of Education, Ocean University of China, Qingdao 266100, China; Laboratory for Marine Ecology and Environmental Science, Qingdao National Laboratory for Marine Science and Technology, Qingdao 266061, China. Electronic address: xinglei@ouc.edu.cn.
  • 6 Key Lab of Submarine Geosciences and Prospecting Techniques, MOE, Qingdao 266100, China.
  • 7 Key Lab of Submarine Geosciences and Prospecting Techniques, MOE, Institute for Advanced Ocean Study, College of Marine Geosciences, Ocean University of China, Qingdao 266100, China.
  • 8 College of Resources and Environment, Chengdu University of Information Technology, Chengdu 610225, China. Electronic address: fsh@cuit.edu.cn.
  • 9 Frontiers Science Center for Deep Ocean Multispheres and Earth System, and Key Laboratory of Marine Chemistry Theory and Technology, Ministry of Education, Ocean University of China, Qingdao 266100, China; Laboratory for Marine Ecology and Environmental Science, Qingdao National Laboratory for Marine Science and Technology, Qingdao 266061, China. Electronic address: baorui@ouc.edu.cn.
  • DOI: 10.1016/j.marpolbul.2023.115931 PMID: 38280293

    摘要 Ai翻译

    Understanding Perfluoroalkyl substances (PFASs) spatial distribution in natural environments is crucial due to their environmental persistence and potential bioaccumulation. However, limited research has investigated PFASs spatial distribution at a high resolution, especially in the Guangdong-Hong Kong-Macao Greater Bay Area. Here, we examined the composition and concentration of PFASs in 36 bulk surface sediments and grain-size fractionated sediments from 9 representative sites to determine the spatial distribution characteristics in Shenzhen Bay. We found that ΣPFASs decreased gradually from nearshore area to offshore area (0.680 and 0.297 ng g-1 dw, respectively). Furthermore, PFASs are easily adsorbed on fine-grained sediments, likely due to their chain length and hydrophobicity. We argue that the lateral movement of sediments may transport fine-grained sediments associated with ΣPFASs out of the bay, resulting in the spatial difference in ΣPFASs in Shenzhen Bay. Our findings provide important insights into explore the mechanisms associated with preservation and transport of PFASs.

    Keywords: Grain size; PFASs; Sediment; Shenzhen Bay; Spatial distribution; Transport mechanism.

    Keywords:perfluoroalkyl substances; spatial distribution; shenzhen bay

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    期刊名:Marine pollution bulletin

    缩写:MAR POLLUT BULL

    ISSN:0025-326X

    e-ISSN:1879-3363

    IF/分区:4.9/Q1

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    Spatial distribution characteristics of perfluoroalkyl substances in bulk and grain size fractionated sediments in Shenzhen Bay