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Multiple-Photon Dynamics in Molecules: A New Approach to High Resolution Spectroscopy of Highly Excited Vibrational States

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Multi-photon transitions with two simultaneously interacting IR laser fields lead to final excited states with frequencies nnu = n1nu1 + n2nu2, with n the total number of photons absorbed and (n, n1, n2) = (2, 1, 1), (3, 2, 1), (4, 1, 3), etc. The nature of th... ...